MULTICOMPONENT DIFFUSION AND REACTION IN COMPOSITE CATALYSTS - A MONTE-CARLO AND DUSTY-GAS MODEL APPROACH APPLIED TO THE METHANOL-TO-OLEFIN SYNTHESIS IN ZEOLITES

Authors

  • Abdul R. Garayhi
  • Frerich J. Keil

Abstract

A model of the description of reaction and mass transport within composite catalysts by Ruckenstein was improved by taking a volume change during the reaction into account, and by describing the internal fluxes by the Dusty-Gas Model. A new numerically improved notation of the Dusty-Gas-Model equations was investigated. The new model is used for describing the Methanol-To-Olefin synthesis in zeolite catalysts. The diffusivities in zeolite particles were obtained by a Monte-Carlo approach. The new model offers an improved description of experimental data.

Keywords:

composite catalysts, dusty-gas model, volume change, zeolites, methanol-to-olefin synthesis

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How to Cite

Garayhi, A. R., Keil, F. J. “MULTICOMPONENT DIFFUSION AND REACTION IN COMPOSITE CATALYSTS - A MONTE-CARLO AND DUSTY-GAS MODEL APPROACH APPLIED TO THE METHANOL-TO-OLEFIN SYNTHESIS IN ZEOLITES ”, Periodica Polytechnica Chemical Engineering, 41(1), pp. 57–72, 1997.

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